To learn Daniel Johnston - Careless Soul chords, anchor your practice on these foundational sequence of chords - C, B, C, B, Ab, F, Ab, B and F. I suggest starting at a calm pace of 42 BPM, and as you gain confidence, approach the song's BPM of 85. For a balanced pitch, adjust the capo with respect to your voice and the song's key: Ab Major.
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Loading chords sheet for Daniel Johnston "Careless Soul" ...