To start learning Simon & Garfunkel - The Sound Of Silence chords, build your understanding on these basic chords - D#m, F#, B, F# and D#m in sequence. A strategic approach would be to train at 56 BPM initially, and then accelerate to the song's tempo of 112. With F# Major as the song's key, tweak the capo to cater to your vocal pitch and chord likes.
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Simon & Garfunkel - Sounds Of Silence/interview/You Can Tell The World/Mr. Tambourine Man (1966)